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We've been there with water damage on a sisal rug. Here's a video that shows how to paint it: https://www.youtube.com/watch?v=bLS0Kf0t9F4
This tutorial explains how to spray paint a sisal rug: https://www.diynetwork.com/how-to/make-and-decorate/decorating/how-to-paint-a-cottage-style-sisal-rug
Yes! You can try using latex wall paint or acrylic artist paint. Both should work well.