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A good primer will stick to almost anything. Maybe try that first.
I second the idea of trying a good primer first!
Silicone is VERY resistant to things adhering... including paint. Try using a fine sandpaper first.
Nail polish remover, rubbing alcohol, Goo Gone, green kitchen scrubby. Sand paper just clogs up.
Are you not able to pull the piece off and try removing the silicone that way? Then just put it back on the wall?